Here are my thoughts. First a crossed effect is an interaction. This means that the effect of one of the terms in the model depends on another term in the model.
You have stumbled upon a significant issue with all quantitative analysis. That is doing quantitative analysis (e.g., ANOVA) prior to analyzing the data for "unusual dat points and patterns" prior to interpreting the results of the quantitative analysis. You should seek to understand why appraiser 2 got different results for UUT #9. I don't see how you conclude consistently, I only see one data point, but none-the-less, why? Within this data set, Deming might call this data point "special" and Shewhart would call it "assignable".
The percentages are of the tolerance. I personally don't think this is the only comparison to judge a measurement system. IMHO, this is the least important as tolerances are independently derived and typically without any insight into the process making the product (or the amount of product variation). What you want your measurement system to be able to do is quantify the variation in the product so that variation may be reduced or predicted. To assess this, you must consider:
1. the discrimination (effective resolution),
2. the stability/consistency,
3. the precision repeatability and perhaps reproducibility,
of the measurement system.
The software is going to want to account for this one unusual data point. Since it is, as you see from the plot, only associated with one appraiser, that would be quantified as an interaction effect (i.e., the effect of appraiser depends on which UUT is measured). Don't be misled by the size of the % (notice the Part variation (UUT) accounts for 720.79 % of tolerance!). You don't have much variation in the appraiser, most of the variation is due to UUT (see the variance component plot).
BTW, one of the issues with crossed studies is that they are usually inadequate for assessing consistency. Control charts don't handle crossed effects. For understanding of consistency, nested studies are preferred.
"All models are wrong, some are useful" G.E.P. Box